A novel dicationic system containing a PN fragment has been synthesized and structurally characterized. According to the solid-state analysis and theoretical investigation, the dicationic iminophosphane resonance form is the most appropriate description for the dication. However, the contribution from the phosphorus mononitride resonance form is not negligible. © 2015 American Chemical Society.

Rakesh Ganguly

SNU Management

Y.K. Loh

C. Gurnani

D. Vidović

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