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A binuclear Cu(ii) complex as an efficient photocatalyst for N-alkylation of aromatic amines
Ranjan R., Chakraborty A., Kyarikwal R., Mukhopadhyay S.,
Published in Royal Society of Chemistry
2022
PMID: 35983724
Volume: 51
   
Issue: 35
Pages: 13288 - 13300
Abstract
Visible-light driven photoreactions using transition metal complexes as catalysts are currently a research hotspot in developing environmentally friendly sustainable processes. To develop a potential copper-based photocatalyst, a binuclear Cu(ii) complex has been synthesized using a Mannich base ligand viz. 2,4-dichloro-6-((4-(2-hydroxyethyl)piperazin-1-yl)methyl)phenol (H2L). The photocatalyst has been characterized using ESI-MS and single crystal X-ray diffraction. Under the irradiation of visible light, the catalyst can catalyze hydrogen auto-transfer in N-alkylated amine formation and benzyl alcohol oxidation reactions with excellent conversion. A plausible mechanistic pathway for catalytic reactions has been explored through ESI-MS spectrometric, UV-Vis spectroscopic and computational studies. © 2022 The Royal Society of Chemistry.
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Published in Royal Society of Chemistry
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